1. Introduction to Reactivity of Carbonyl Group
  • The carbonyl group (C=O) is a highly reactive functional group found in aldehydes and ketones.
  • Understanding the reactivity of the carbonyl group is crucial in organic chemistry.
  • The reactivity of carbonyl compounds can be influenced by various factors.
  1. Nucleophilic Addition Reactions
  • Nucleophiles are electron-rich species that can attack and form a covalent bond with the carbonyl carbon.
  • Addition reactions occur when a nucleophile adds to the carbonyl group, resulting in the formation of a new compound.
  • Examples of nucleophilic addition reactions include:
    • Addition of water (hydration)
    • Addition of alcohols
    • Addition of amines
  1. Hydration of Carbonyl Compounds
  • Aldehydes and ketones can undergo hydration in the presence of water and an acid catalyst.
  • The carbonyl group is converted into a geminal diol, or hydrate.
  • The reaction is reversible and can be influenced by the reaction conditions.
  1. Addition of Alcohols (Hemiacetals and Acetals)
  • Aldehydes and ketones can react with alcohols to form hemiacetals and acetals.
  • Hemiacetals are formed when one alcohol molecule adds to the carbonyl group, resulting in the formation of a new alcohol functional group.
  • Acetals are formed when two alcohol molecules add to the carbonyl group.
  • The reaction is reversible and can be influenced by the reaction conditions.
  1. Addition of Amines (Imine and Enamine Formation)
  • Aldehydes and ketones can react with primary amines to form imines.
  • Imines are formed when the amino group adds to the carbonyl group.
  • Secondary amines can react with ketones to form enamines.
  • The reaction is reversible and can be influenced by the reaction conditions.
  1. Oxidation Reactions of Carbonyl Compounds
  • Aldehydes can be further oxidized to carboxylic acids.
  • The oxidation can be accomplished using mild oxidizing agents such as Tollens’ reagent or Fehling’s solution.
  • The reaction involves the conversion of the aldehyde into a carboxylate ion.
  • Ketones, on the other hand, are resistant to oxidation under normal conditions.
  1. Reduction Reactions of Carbonyl Compounds
  • Carbonyl compounds can be reduced to alcohols using reducing agents such as sodium borohydride (NaBH4) or lithium aluminum hydride (LiAlH4).
  • The reduction process involves the addition of hydrogen atoms to the carbonyl carbon, resulting in the formation of an alcohol functional group.
  1. Reactivity of Aldehydes and Ketones towards Nucleophiles
  • Aldehydes are generally more reactive than ketones towards nucleophilic addition reactions.
  • This is because aldehydes have a less sterically hindered carbonyl group compared to ketones.
  • Additionally, the electron-withdrawing effect of alkyl groups in ketones makes them less reactive.
  1. Reactivity of Aldehydes and Ketones towards Strong Nucleophiles
  • Aldehydes and ketones can react with strong nucleophiles like Grignard reagents (RMgX) or organolithium compounds (RLi).
  • The addition of the nucleophile to the carbonyl group forms a new carbon-carbon bond.
  • The reaction proceeds through the formation of a highly reactive alkoxide ion intermediate.
  1. Reactivity of Aldehydes and Ketones towards Oxidizing Agents
  • Aldehydes and ketones can react with oxidizing agents like chromic acid (H2CrO4) or potassium permanganate (KMnO4).
  • The reaction results in the oxidation of the carbonyl compound to a carboxylic acid.
  • Aldehydes are easily oxidized, while ketones require stronger oxidizing conditions.
  1. Reactivity of Aldehydes and Ketones towards Reduction
  • Aldehydes and ketones can be reduced to alcohols using various reducing agents.
  • Sodium borohydride (NaBH4) is commonly used as a mild reducing agent for this purpose.
  • The reaction mechanism involves the transfer of a hydride ion (H-) to the carbonyl carbon, resulting in the formation of an alcohol.
  • Example:
    • Reduction of acetone (a ketone) with NaBH4 yields isopropyl alcohol.
  1. Reactivity of Aldehydes and Ketones towards Grignard Reagents
  • Aldehydes and ketones can react with Grignard reagents (RMgX) to form alcohols.
  • The reaction involves the addition of the nucleophilic carbon of the Grignard reagent to the carbonyl carbon.
  • The resulting alkoxide ion (RO-) is converted to an alcohol after acidic work-up.
  • Example:
    • Reaction of propanal (an aldehyde) with methylmagnesium bromide (CH3MgBr) yields 2-methylpropan-2-ol.
  1. Reactivity of Aldehydes and Ketones towards Cyanide Ion
  • Aldehydes and ketones can react with cyanide ion (CN-) to form cyanohydrins.
  • The nucleophilic addition of CN- to the carbonyl carbon followed by protonation yields the product.
  • Cyanohydrins are important intermediates in organic synthesis.
  • Example:
    • Reaction of propanal with sodium cyanide (NaCN) yields 2-hydroxypropanenitrile.
  1. Reactivity of Aldehydes and Ketones towards Wolff-Kishner Reduction
  • Aldehydes and ketones can undergo Wolff-Kishner reduction to form alkanes.
  • The reaction involves the conversion of the carbonyl group to a methylene group (-CH2-) using hydrazine (H2NNH2) and a strong base.
  • The resulting hydrazone is then thermally decomposed to yield the alkane.
  • Example:
    • Reduction of acetophenone using Wolff-Kishner conditions gives ethylbenzene.
  1. Reactivity of Aldehydes and Ketones towards Clemmensen Reduction
  • Aldehydes and ketones can undergo Clemmensen reduction to form alkanes.
  • The Clemmensen reduction involves the reduction of the carbonyl group to a methylene group using amalgamated zinc (Zn(Hg)) and hydrochloric acid (HCl).
  • The reaction proceeds through the formation of an organozinc intermediate, followed by elimination of the carbonyl oxygen.
  • Example:
    • Reduction of benzaldehyde using Clemmensen conditions gives toluene.
  1. Reactivity of Aldehydes and Ketones towards Nitrogen Compounds
  • Aldehydes and ketones can react with nitrogen compounds to form a variety of products.
  • Amines can add to the carbonyl group to form imines or enamines, depending on the nitrogen compound used.
  • Hydrazines can react with aldehydes and ketones to form hydrazones.
  • Example:
    • Reaction of acetone with phenylhydrazine yields phenylhydrazone.
  1. Reactivity of Aldehydes and Ketones towards Organometallic Compounds
  • Aldehydes and ketones can react with organometallic compounds such as Grignard reagents and organolithium compounds.
  • The carbon-metal bond in the organometallic compound adds to the carbonyl carbon, resulting in the formation of a new carbon-carbon bond.
  • The reaction is widely used in organic synthesis.
  • Example:
    • Reaction of benzaldehyde with phenylmagnesium bromide (PhMgBr) gives 1-phenylethanol.
  1. Reactivity of Aldehydes and Ketones towards Ammonia Derivatives
  • Aldehydes and ketones can react with ammonia derivatives such as hydroxylamine, semicarbazide, and phenylhydrazine.
  • These reactions are used for the identification and characterization of carbonyl compounds.
  • Example:
    • Reaction of acetone with phenylhydrazine yields 2,4-dinitrophenylhydrazone.
  1. Reactivity of Aldehydes and Ketones towards Oxidizing Agents
  • Aldehydes can be easily oxidized to carboxylic acids using oxidizing agents such as potassium permanganate (KMnO4) or chromic acid (H2CrO4).
  • Ketones, on the other hand, are resistant to oxidation under normal conditions.
  • Example:
    • Oxidation of ethanol (an aldehyde) using KMnO4 yields acetic acid.
  1. Summary of Reactivity of Carbonyl Group
  • Aldehydes and ketones exhibit a wide range of reactivity towards different nucleophiles and oxidizing agents.
  • The reactivity can be influenced by factors such as the size of the carbonyl group, the presence of electron-donating or withdrawing groups, and the nature of the nucleophile or oxidizing agent.
  • Understanding the reactivity of carbonyl compounds is essential for the synthesis and functionalization of organic molecules.

Problem Solving Session Aldehydes And Ketones - Reactivity of carbonyl group

Slide 21:

  1. Problem:
    • Predict the major product formed when propanal reacts with methanol in the presence of an acid catalyst.
  1. Solution:
    • Propanal reacts with methanol to form a hemiacetal.
    • The oxygen of the carbonyl group attacks the hydrogen of the alcohol, and the alcohol oxygen becomes protonated.
    • Example:
      • CH3CH2CHO + CH3OH → CH3CH(OMe)OH
  1. Problem:
    • Predict the major product formed when butanone reacts with phenylmagnesium bromide.
  1. Solution:
    • Butanone reacts with phenylmagnesium bromide to form a tertiary alcohol.
    • The carbon of the phenyl group in the Grignard reagent adds to the carbon of the carbonyl group.
    • Example:
      • CH3COCH2CH3 + PhMgBr → CH3COCH2CH2Ph
  1. Problem:
    • Predict the major product formed when acetone reacts with hydrogen cyanide.
  1. Solution:
    • Acetone reacts with hydrogen cyanide to form a cyanohydrin.
    • The nucleophilic cyanide ion attacks the carbonyl carbon, resulting in the formation of a new carbon-carbon bond.
    • Example:
      • CH3COCH3 + HCN → CH3CH(OH)CN
  1. Problem:
    • Predict the major product formed when benzaldehyde reacts with phenylhydrazine.
  1. Solution:
    • Benzaldehyde reacts with phenylhydrazine to form a phenylhydrazone.
    • The hydrazine nitrogen acts as a nucleophile and attacks the carbonyl carbon.
    • Example:
      • C6H5CHO + C6H5NHNH2 → C6H5CH=N-NHC6H5
  1. Problem:
    • Predict the major product formed when propanal reacts with NaBH4.
  1. Solution:
    • Propanal reacts with sodium borohydride (NaBH4) to form a primary alcohol.
    • The hydride ion (H-) reduces the carbonyl group, resulting in the formation of an alcohol.
    • Example:
      • CH3CH2CHO + NaBH4 → CH3CH2CH2OH

Slide 22:

  1. Problem:
    • Predict the major product formed when butanone is oxidized using chromic acid (H2CrO4).
  1. Solution:
    • Butanone can be oxidized to butanoic acid using chromic acid (H2CrO4) as an oxidizing agent.
    • The carbonyl group is converted into a carboxylic acid.
    • Example:
      • CH3COCH2CH3 + H2CrO4 → CH3COCH2COOH
  1. Problem:
    • Predict the major product formed when 2-propanol is oxidized using potassium permanganate (KMnO4).
  1. Solution:
    • 2-Propanol can be oxidized to acetone using potassium permanganate (KMnO4) as an oxidizing agent.
    • The primary alcohol is converted into a ketone.
    • Example:
      • CH3CH(OH)CH3 + KMnO4 → CH3COCH3
  1. Problem:
    • Predict the major product formed when benzaldehyde is reduced using sodium borohydride (NaBH4).
  1. Solution:
    • Benzaldehyde can be reduced to benzyl alcohol using sodium borohydride (NaBH4) as a reducing agent.
    • The carbonyl group is reduced to an alcohol.
    • Example:
      • C6H5CHO + NaBH4 → C6H5CH2OH
  1. Problem:
    • Predict the major product formed when butanone is reduced using lithium aluminum hydride (LiAlH4).
  1. Solution:
    • Butanone can be reduced to 2-butanol using lithium aluminum hydride (LiAlH4) as a reducing agent.
    • The carbonyl group is reduced to an alcohol.
    • Example:
      • CH3COCH2CH3 + LiAlH4 → CH3CH(OH)CH2CH3
  1. Problem:
    • Predict the major product formed when acetone reacts with methylmagnesium bromide.
  1. Solution:
    • Acetone reacts with methylmagnesium bromide (CH3MgBr) to form 2-methylpropan-2-ol.
    • The methyl group of the Grignard reagent adds to the carbonyl carbon.
    • Example:
      • CH3COCH3 + CH3MgBr → (CH3)2C(OH)CH3

Slide 23:

  1. Problem:
    • Predict the major product formed when propanal is reacted with semicarbazide in the presence of an acid catalyst.
  1. Solution:
    • Propanal reacts with semicarbazide to form a semicarbazone.
    • The -NH2 group of the semicarbazide acts as a nucleophile and attacks the carbonyl carbon.
    • Example:
      • CH3CH2CHO + H2NNHC(O)NH2 → CH3CH2CH=N-NHCONH2
  1. Problem:
    • Predict the major product formed when benzaldehyde is reacted with hydrazine in the presence of an acid catalyst.
  1. Solution:
    • Benzaldehyde reacts with hydrazine to form a phenylhydrazone.
    • The -NH2 group of the hydrazine acts as a nucleophile and attacks the carbonyl carbon.
    • Example:
      • C6H5CHO + H2NNH2 → C6H5CH=N-NH2
  1. Problem:
    • Predict the major product formed when propanal is reacted with Grignard reagent (CH3CH2MgBr).
  1. Solution:
    • Propanal reacts with the Grignard reagent (CH3CH2MgBr) to form 3-hexanol.
    • The carbon of the Grignard reagent adds to the carbonyl carbon.
    • Example:
      • CH3CH2CHO + CH3CH2MgBr → CH3(CH2)3OH
  1. Problem:
    • Predict the major product formed when butanone is reacted with lithium diisopropylamide (LDA).
  1. Solution:
    • Butanone reacts with lithium diisopropylamide (LDA) to form an enolate ion.
    • The deprotonated LDA attacks the carbonyl carbon, leading to enol formation followed by tautomeric shift.
    • Example:
      • CH3COCH2CH3 + LDA → CH3COCH=C(CH3)2
  1. Problem:
    • Predict the major product formed when acetone is reacted with nitrous acid (HNO2).
  1. Solution:
    • Acetone reacts with nitrous acid (HNO2) to form an oxime.
    • The -OH group of the nitrous acid acts as a nucleophile and attacks the carbonyl carbon.
    • Example:
      • CH3COCH3 + HNO2 → CH3C(NOH)CH3

Slide 24:

  1. Problem:
    • Predict the major product formed when propanal reacts with methylamine.
  1. Solution:
    • Propanal reacts with methylamine to form an imine.
    • The -NH2 group of methylamine acts as a nucleophile and attacks the carbonyl carbon.
    • Example:
      • CH3CH2CHO + CH3NH2 → CH3CH2CH=NCH3
  1. Problem:
    • Predict the major product formed when butanone reacts with ethylamine.
  1. Solution:
    • Butanone reacts with ethylamine to form an imine.
    • The -NH2 group of ethylamine acts as a nucleophile and attacks the carbonyl carbon.
    • Example:
      • CH3COCH2CH3 + C2H5NH2 → CH3COCH2CH=NH2
  1. Problem:
    • Predict the major product formed when acetone reacts with ethylene glycol in the presence of an acid catalyst.
  1. Solution:
    • Acetone reacts with ethylene glycol to form a ketal.
    • The oxygen of the carbonyl group attacks the hydrogen of the alcohol, and the alcohol oxygen becomes protonated.
    • Example:
      • CH3COCH3 + HOCH2CH2OH →